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New paper published in ACS Energy Letters on selective lithium-ion extraction with interlayer-modified MXene

New paper published in ACS Energy Letters on interlayer-tailored Alkyl-MXenes for selective electrochemical lithium-ion extraction. The paper reports a two-step electrochemical lithium-ion extraction strategy using interlayer-tailored Ti3C2Tx MXene electrodes. By pre-intercalating long-chain organic molecules (hexadecylamine, HDA, and decyltrimethylammonium, C10), the MXene interlayer environment is tuned to favor Li+ over competing Na+, improving both selectivity and extraction rates. In the demonstrated conditions, the HDA-intercalated MXene shows 2.2 mmol/L Li uptake with suppressed Na uptake (<0.2 mmol/L), and both HDA-Ti3C2Tx and C10-Ti3C2Tx maintain nearly 100% lithium purity over 50 cycles. Co-authors: Cansu Kök, Karamullah Eisawi, Jean G. A. Ruthes, Burcu Tan, Antje Quade, Michael Naguib. We are grateful to be featured on the Supporting Cover.